Radiative Double Electron Capture (RDEC) of Ions with Quasi-Free Electrons

Western Michigan University, Kalamazoo MI

Investigators

Abstract

Non-technical description: This project involves an investigation of how two of the smallest and most fundamental constituents of matter (electrons) exchange information with each other (the analog of "talking") when they are transferred from one atom to another as the two atoms move by each other quickly. In the process to be studied, the two electrons come from a target atom and are captured by a fast moving projectile ion (an atom missing some electrons on it initially) accompanied by the emission of a single x ray. The process can be thought of as the inverse of the double ionization (removal of two electrons) by a single photon. This two-electron process is similar to the one-electron process in which an electron is liberated by a single photon. The latter process is known as the photoelectric effect, which was explained by Einstein in 1905, for which he was awarded the Nobel Prize, and which underlies much of modern technology. During the two-electron process the electrons "talk" with each other and coordinate the double photo-ionization. The same must occur in the time-reversed case when two electrons are transferred to a projectile, giving up a photon. There is considerable interest in studying this "talking" process, from the point of view of collisions between ions and target atoms and from the time-reversed process of double photo-ionization of an atom by a single photon. Theorists have calculated probabilities for the two-electron process, with results differing by factors of 1,000 or even 10,000. This wide range leaves the field open for experiments that will determine the actual probability accurately. Up to now, five experiments of two-electron transfer with simultaneous emission of a photon have been attempted at laboratories in the U.S. and Germany. One of these experiments (in the U.S.) was partially successful, but the others were not, mostly due to the long measuring times required to see the events. Notably, photon collision researchers would be very much interested in measuring double photo-ionization of two-electron ions, something they cannot yet do, except for the two-electron atom helium. The involvement of Ph.D. students in the planned research gives them valuable training in state-of-the-art physics experiments, and along with the preparation of collaborative manuscripts and abstracts, help make them productive young scientists. Technical description: The transfer of two electrons to an ion accompanied by the emission of a single photon is called radiative-double-electron capture, or RDEC for short. The intellectual merit of RDEC lies in its intrinsic fundamental interest in the field of ion collisions with quasi-free electrons, and its close relationship to photon interactions with highly-charged ions. This relationship is essentially the time inverse of RDEC, which is the process of double photo-ionization of ions. These inverse processes are particularly connected when RDEC occurs for incident fully-stripped ions and double photo-ionization for two-electron systems. RDEC has been investigated sparsely, and new studies will address complications of the previous data involving ion-solid interactions for oxygen and fluorine ions incident on a C foil, and will build upon these results by investigating RDEC for collisions with gas targets of He, N2 and Ne. An advantage of gas targets is that they do not introduce the effects of multiple collisions present for solid targets and the results are expected to clarify the questions that arose in the earlier work. RDEC can be compared with several theoretical calculations that differ by several orders of magnitude. By obtaining results for C-foil targets and for gas targets, both to be studied under this project, and by comparing the measurements with theory, it should be possible to obtain the first data that provides input to the theoretical calculations. The measurements will be done for fully-stripped fluorine ions using the tandem Van de Graaff at Western Michigan University. The particular apparatus for the proposed experiment, including the apparatus for the gaseous targets, is already in place (funded previously by the US DOE). Measurements will involve recording coincidences between x rays emitted and singly- and doubly-charged projectiles (the latter coincidences represent a signature for RDEC). The measurements are difficult due to the relatively small cross sections for RDEC (on the order of ~1 barn or less) and will require long counting times of more than a month.